The rest of the characters can be unlocked by completing Time Attack (under CPU Battles) with specific characters:
(Character) -> (Unlockable)
Genryusai -> Komamura
Komamura -> Hisagi
Ukitake -> Kyoraku
Kyoraku -> Nanao
Kenpachi -> Yachiru
Mayuri -> Nemu
Rukia -> Shinigami Rukia
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